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Interfacial Processes in Lithium-Ion Batteries Using Advanced Characterization

Delft University of Technology Faculty of Applied Sciences
Self-funded ⏰ Closing Soon 🎓 Chemical Engineering 🎓 Materials Science 🎓 Physics atomic layer deposition materials characterization solid electrolyte interphase cathode electrolyte interphase lithium-ion batteries pfas-free electrolyte electrochemical testing fib-sem

Explore interfacial chemistry in lithium-ion batteries focusing on SEI and CEI formation using advanced characterization. Develop insights into optimizing formation protocols with ALD coatings and environmentally friendly electrolytes to improve battery efficiency and safety.

AI-generated overview

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Why This Research Matters

This research addresses critical challenges in lithium-ion battery technology by investigating and optimizing interphase formation, which can reduce production costs and enhance battery performance and safety. The societal benefit includes advancing sustainable and safer energy storage solutions pivotal for electric vehicles and renewable energy integration.

Energy Storage Li-ion batteries Li-air batteries

Project Description

Project Overview

This project is part of the DigiCellFab initiative aiming to develop a fundamental understanding of the formation and stabilization of the Solid Electrolyte Interphase (SEI) and Cathode Electrolyte Interphase (CEI) in lithium-ion batteries. The work focuses on reducing production time and cost while improving battery performance and safety by optimizing formation protocols and using Atomic Layer Deposition (ALD)-based protective coatings to control interphase formation.

What You Will Do

The PhD candidate will systematically study the interplay between formation conditions (such as current density, temperature, pressure), electrolyte composition, and coated electrode surfaces with an emphasis on using PFAS-free electrolyte systems. The research involves combining electrochemical testing with advanced characterization techniques like FIB-SEM for site-specific cross-sectioning and interphase analysis, supported by complementary microscopy and spectroscopy methods.

Expected Outcomes

The project aims to establish direct structure-function relationships linking formation protocols, coating properties, and interphase characteristics to battery performance, offering pathways to more sustainable, cost-effective, and safer lithium-ion batteries.

Why This Matters

Understanding and controlling the nanoscale interphase layers in lithium-ion batteries is crucial to enhancing their longevity, safety, and environmental footprint. This research contributes to advancing energy storage technology critical for sustainable energy solutions worldwide.

Entry Requirements

A Master’s degree in Chemistry, Materials Science, Chemical Engineering, Physics, or a closely related field. Solid understanding of electrochemistry and/or materials characterization. Interest in interfacial phenomena in batteries, particularly SEI/CEI formation. Experience with electrochemical and/or advanced characterization methods is advantageous. Hands-on experimental skills are required.

Eligibility

UK/Home
EU
International

Supervisor Profile

DS
Dr. Swapna Ganapathy
Delft University of Technology, Faculty of Applied Sciences

Dr. Swapna Ganapathy is a researcher affiliated with the Faculty of Applied Sciences at Delft University of Technology, focusing on battery materials and interfacial phenomena. Her work involves advanced characterization of electrochemical systems, particularly the nanoscale processes governing battery performance and stability. She contributes to collaborative projects like DigiCellFab, aiming to innovate lithium-ion battery technology.

Key Publications

2019 742 citations
Review of recent development of in situ/operando characterization techniques for lithium battery research
2020 574 citations
Clarifying the relationship between redox activity and electrochemical stability in solid electrolytes
2017 461 citations
Accessing the bottleneck in all-solid state batteries, lithium-ion transport over the solid-electrolyte-electrode interface
2020 446 citations
Revealing high Na-content P2-type layered oxides as advanced sodium-ion cathodes
2024 410 citations
Origin of fast charging in hard carbon anodes

Research Contributions

Developed in situ and operando characterization techniques for lithium battery research.
Enabled deeper understanding of battery chemistry and mechanisms, improving battery performance and design.
Investigated lithium-ion transport across solid-electrolyte-electrode interfaces in all-solid-state batteries.
Addressed critical transport bottlenecks to enhance the efficiency and viability of solid-state batteries.
Explored high sodium-content layered oxides as advanced cathode materials for sodium-ion batteries.
Contributed to the development of cost-effective and sustainable sodium-ion energy storage solutions.
Clarified the relationship between redox activity and electrochemical stability in solid electrolytes.
Provided guidance for designing more stable and efficient solid-state electrolytes for battery applications.

More PhDs with Dr. Swapna Ganapathy

Interfacial Processes in Lithium-Ion Batteries Using Advanced Characterization
Delft University of Technology Dr. Swapna Ganapathy 🎓 Chemical Engineering 🎓 Chemistry Deadline: 17 May 2026

Explore how interfacial layers in lithium-ion batteries affect their performance and stability. Use cutting-edge techniques like FIB-SEM alongside electrochemical testing to innovate safer, cost-effective battery techno…

This research addresses key challenges in lithium-ion battery technology by optimizing protective coatings and formation protocols, which c…

Energy Storage Li-ion batteries Li-air batteries

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