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Interfacial Processes in Lithium-Ion Batteries Using Advanced Characterization

Delft University of Technology Faculty of Applied Sciences
✓ Fully Funded ⏰ Closing Soon 🎓 Chemical Engineering 🎓 Chemistry 🎓 Materials Science atomic layer deposition solid electrolyte interphase cathode electrolyte interphase lithium-ion batteries electrochemical testing fib-sem battery safety pfas-free electrolytes

Explore how interfacial layers in lithium-ion batteries affect their performance and stability. Use cutting-edge techniques like FIB-SEM alongside electrochemical testing to innovate safer, cost-effective battery technologies with environmentally friendly electrolytes.

AI-generated overview

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Why This Research Matters

This research addresses key challenges in lithium-ion battery technology by optimizing protective coatings and formation protocols, which can lead to safer, longer-lasting batteries with reduced production costs. Employing PFAS-free electrolytes also contributes to making batteries more environmentally sustainable, supporting the transition to greener energy solutions.

Energy Storage Li-ion batteries Li-air batteries

Project Description

Project Overview

This PhD focuses on the fundamental understanding of Solid Electrolyte Interphase (SEI) and Cathode Electrolyte Interphase (CEI) formation in lithium-ion batteries. It aims to optimize formation protocols to reduce production time and cost while improving battery performance and safety. The role of Atomic Layer Deposition (ALD) based protective coatings in controlling interphase formation and stabilizing electrode-electrolyte interfaces is central to the research.

What You Will Do

The research involves systematically investigating the interplay among formation conditions (e.g., current density, temperature, pressure), electrolyte composition, and coated electrode surfaces. It emphasizes the use of PFAS-free electrolyte systems. You will combine electrochemical testing with advanced characterization techniques including FIB-SEM for site-specific cross-sectioning and interphase analysis, supported by complementary microscopy and spectroscopic methods. The aim is to establish direct structure-function relationships linking formation protocols, coating properties, and interphase characteristics to battery performance.

Expected Outcomes

The project aims to develop optimized formation protocols and coating strategies that enhance lithium-ion battery stability, safety, and performance with reduced production costs and times. The direct correlations established between structure and function will enable advanced battery designs.

Why This Matters

Improved understanding and control of interphase layers in batteries are critical for developing safer, longer-lasting, and more sustainable energy storage solutions. This research supports the transition to cleaner technologies by advancing lithium-ion battery performance and reducing environmental impact through PFAS-free electrolytes.

Entry Requirements

Master’s degree in Chemistry, Materials Science, Chemical Engineering, Physics, or a closely related field with a solid understanding of electrochemistry and/or materials characterization. Experience with electrochemical techniques or advanced characterization methods is advantageous.

Eligibility

UK/Home
EU
International

Supervisor Profile

DS
Dr. Swapna Ganapathy
Delft University of Technology, Faculty of Applied Sciences

Dr. Swapna Ganapathy is a researcher specializing in interfacial processes and advanced characterization techniques for battery materials. Her work focuses on understanding and controlling the nanoscale interfaces in lithium-ion batteries to enhance performance, safety, and sustainability. She is recognized for integrating electrochemical methods with microscopy and spectroscopy to study battery interphases.

Key Publications

2019 743 citations
Review of recent development of in situ/operando characterization techniques for lithium battery research
2020 575 citations
Clarifying the relationship between redox activity and electrochemical stability in solid electrolytes
2017 462 citations
Accessing the bottleneck in all-solid state batteries, lithium-ion transport over the solid-electrolyte-electrode interface
2020 446 citations
Revealing high Na-content P2-type layered oxides as advanced sodium-ion cathodes
2024 413 citations
Origin of fast charging in hard carbon anodes

Research Contributions

Development and application of in situ/operando characterization techniques for lithium battery research.
Advances understanding of battery material behavior during operation, aiding in battery design and performance optimization.
Investigation of lithium-ion transport at solid-electrolyte-electrode interfaces in all-solid state batteries.
Addresses bottlenecks in battery performance, contributing to enhanced solid-state battery efficiency and durability.
Exploration of sodium-ion cathodes and their high Na-content layered oxide structures.
Supports the development of advanced sodium-ion batteries as alternatives to lithium-ion technologies.
Elucidation of fast charging mechanisms in hard carbon anodes.
Enables design of batteries with faster charging capabilities, improving usability and consumer experience.

More PhDs with Dr. Swapna Ganapathy

Interfacial Processes in Lithium-Ion Batteries Using Advanced Characterization
Delft University of Technology Dr. Swapna Ganapathy 🎓 Chemical Engineering 🎓 Materials Science Deadline: 17 May 2026

Explore interfacial chemistry in lithium-ion batteries focusing on SEI and CEI formation using advanced characterization. Develop insights into optimizing formation protocols with ALD coatings and environmentally friend…

This research addresses critical challenges in lithium-ion battery technology by investigating and optimizing interphase formation, which c…

Energy Storage Li-ion batteries Li-air batteries

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